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Correcting an Error in Some Interpretations of Atmospheric 14C Data

Received: 5 July 2020    Accepted: 4 August 2020    Published: 13 August 2020
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Abstract

The variable “∆14C”, commonly used in radiocarbon dating and tracing applications to quantify 14C levels, is a measure of the ratio of the radioisotope 14C to other carbon in a sample. After atmospheric nuclear testing in the 1950’s and 1960’s nearly doubled atmospheric 14C, the later evolution of ∆14C allowed insights into the dynamics of carbon exchange between the atmosphere and terrestrial and marine sinks. But a few authors without backgrounds in isotope measurements have confused ∆14C with excess 14C concentration. They erroneously interpret the present recovery of ∆14C to near its pre bomb test value as evidence that atmospheric 14C concentration has returned to its earlier value. From this they reach further incorrect conclusions about the fate of anthropogenic CO2 introduced into the atmosphere by fossil fuel burning. An estimate of the true time dependence of atmospheric 14C concentration over the past century, calculated from averaged atmospheric ∆14C and CO2 data is presented. The data show that 14C concentrations remain over 30% above 1950 values, and have begun to increase, even as ∆14C continues to fall. This confirms the prediction of a conventional model of the carbon cycle. The unconventional models of carbon dynamics motivated by the mistake, on the other hand, are excluded by the properly interpreted 14C data.

Published in Earth Sciences (Volume 9, Issue 4)
DOI 10.11648/j.earth.20200904.12
Page(s) 126-129
Creative Commons

This is an Open Access article, distributed under the terms of the Creative Commons Attribution 4.0 International License (http://creativecommons.org/licenses/by/4.0/), which permits unrestricted use, distribution and reproduction in any medium or format, provided the original work is properly cited.

Copyright

Copyright © The Author(s), 2024. Published by Science Publishing Group

Keywords

Carbon Accumulation, Radiocarbon, Atmospheric CO2

References
[1] Essenhigh, R. H. (2009). Potential dependence of global warming on the residence time (RT) in the atmosphere of anthropogenically sourced carbon dioxide. Energy & Fuels, 23, 2773−2784.
[2] Harde, H.(2017). Scrutinizing the carbon cycle and CO2 residence time in the atmosphere. Global and Planetary Change, 152, 19-26.
[3] Harde, H. (2019). What humans contribute to atmospheric CO2: Comparison of carbon cycle models with observations. Earth Sciences. 8 (3), 139-159. doi: 10.11648/j.earth.20190803.13.
[4] Berry, E. X. (2019). Human CO2 emissions have little effect on atmospheric CO2. International Journal of Atmospheric and Oceanic Sciences, 3 (1), 13-26. doi: 10.11648/j.ijaos.20190301.13.
[5] Cawley, G. C. (2011). On the atmospheric residence time of anthropogenically sourced CO2. Energy Fuels 25, 5503–5513, http://dx.doi.org/10.1021/ef200914u.
[6] Koehler, P., Hauck, J., Volker, C,. Wolf-Gladrow, D. A., Butzin, M, Halpern, J. B. et al.(2017) Comment on “Scrutinizing the carbon cycle and CO2 residence time in the atmosphere by H. Harde”. Global and Planetary Change. 164, 67-71.
[7] Caldeira, K., Raul, G. H., and Duffy, P. B. (1998). Predicted net efflux of radiocarbon from the ocean and increase in atmospheric radiocarbon content. Geophysical Research Letters, 25 (20), 3811-3814.
[8] Turnbull, J., Rayne, P., Miller, J., Naegler, T., Ciais, P., Cozic, A. (2009). On the use of 14CO2 as a tracer for fossil fuel CO2: Quantifying uncertainties using an atmospheric transport model., Journal of Geophysical Research, 114, D22302. https://doi.org/10.1029/2009JD012308
[9] Levin, I. and Hesshaimer, V. (2000). Radiocarbon: A unique tracer of global carbon cycle dynamics., Radiocarbon, 42 (1), 69–80.
[10] Turnbull, J. C., Mikaloff Fletcher, S. E., Ansell, I., Brailsford, G. W, Moss, R. C., Norris, M. W, et al. (2017). Sixty years of radiocarbon dioxide measurements at Wellington, New Zealand: 1954–2014. Atmos. Chem. Phys., 17, 14771–14784. https://doi.org/10.5194/acp-17-14771-2017.
[11] Hua, Q., Barbetti, M., Rakowski, A. Z. (2013). Atmospheric radiocarbon for the period 1950–2010. Radiocarbon, 55, pp. 2059–2072. https://doi.org/10.2458/azu_js_rc.v55i2.16177
[12] Graven, H., Allison, C. E., Etheridge, D. M., Hammer, S., Keeling, R. F., Levin, I., et al. (2017). Compiled records of carbon isotopes in atmospheric CO2 for historical simulations in CMIP6, Geosci. Model Dev., 10, 4405–4417, https://doi.org/10.5194/gmd-10-4405-2017.
[13] Stenstrom, K. E., Skog, G., Gerogiadou, Genberg. J., Johansson, A. (2011). A guide to radiocarbon units and calculations. Lund University, LUNFD6 (NFFR-3111) /1-17/ (2011). https://www.hic.ch.ntu.edu.tw/AMS/A%20guide%20to%20radiocarbon%20units%20and%20calculations.pdf
[14] Stuiver, M. and Polach, H.(1977). Discussion: Reporting of 14C data”. Radiocarbon, 19 (3), 355-363. https://journals.uair.arizona.edu/index.php/radiocarbon/article/viewFile/493/498
[15] World Data Centre for Greenhouse Gasses http://gaw.kishou.go.jp/
[16] Suess, H. E. (1955), Radiocarbon concentration in modern wood”, Science, 122, 415-417.
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    David Evans Andrews. (2020). Correcting an Error in Some Interpretations of Atmospheric 14C Data. Earth Sciences, 9(4), 126-129. https://doi.org/10.11648/j.earth.20200904.12

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    ACS Style

    David Evans Andrews. Correcting an Error in Some Interpretations of Atmospheric 14C Data. Earth Sci. 2020, 9(4), 126-129. doi: 10.11648/j.earth.20200904.12

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    AMA Style

    David Evans Andrews. Correcting an Error in Some Interpretations of Atmospheric 14C Data. Earth Sci. 2020;9(4):126-129. doi: 10.11648/j.earth.20200904.12

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  • @article{10.11648/j.earth.20200904.12,
      author = {David Evans Andrews},
      title = {Correcting an Error in Some Interpretations of Atmospheric 14C Data},
      journal = {Earth Sciences},
      volume = {9},
      number = {4},
      pages = {126-129},
      doi = {10.11648/j.earth.20200904.12},
      url = {https://doi.org/10.11648/j.earth.20200904.12},
      eprint = {https://article.sciencepublishinggroup.com/pdf/10.11648.j.earth.20200904.12},
      abstract = {The variable “∆14C”, commonly used in radiocarbon dating and tracing applications to quantify 14C levels, is a measure of the ratio of the radioisotope 14C to other carbon in a sample. After atmospheric nuclear testing in the 1950’s and 1960’s nearly doubled atmospheric 14C, the later evolution of ∆14C allowed insights into the dynamics of carbon exchange between the atmosphere and terrestrial and marine sinks. But a few authors without backgrounds in isotope measurements have confused ∆14C with excess 14C concentration. They erroneously interpret the present recovery of ∆14C to near its pre bomb test value as evidence that atmospheric 14C concentration has returned to its earlier value. From this they reach further incorrect conclusions about the fate of anthropogenic CO2 introduced into the atmosphere by fossil fuel burning. An estimate of the true time dependence of atmospheric 14C concentration over the past century, calculated from averaged atmospheric ∆14C and CO2 data is presented. The data show that 14C concentrations remain over 30% above 1950 values, and have begun to increase, even as ∆14C continues to fall. This confirms the prediction of a conventional model of the carbon cycle. The unconventional models of carbon dynamics motivated by the mistake, on the other hand, are excluded by the properly interpreted 14C data.},
     year = {2020}
    }
    

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  • TY  - JOUR
    T1  - Correcting an Error in Some Interpretations of Atmospheric 14C Data
    AU  - David Evans Andrews
    Y1  - 2020/08/13
    PY  - 2020
    N1  - https://doi.org/10.11648/j.earth.20200904.12
    DO  - 10.11648/j.earth.20200904.12
    T2  - Earth Sciences
    JF  - Earth Sciences
    JO  - Earth Sciences
    SP  - 126
    EP  - 129
    PB  - Science Publishing Group
    SN  - 2328-5982
    UR  - https://doi.org/10.11648/j.earth.20200904.12
    AB  - The variable “∆14C”, commonly used in radiocarbon dating and tracing applications to quantify 14C levels, is a measure of the ratio of the radioisotope 14C to other carbon in a sample. After atmospheric nuclear testing in the 1950’s and 1960’s nearly doubled atmospheric 14C, the later evolution of ∆14C allowed insights into the dynamics of carbon exchange between the atmosphere and terrestrial and marine sinks. But a few authors without backgrounds in isotope measurements have confused ∆14C with excess 14C concentration. They erroneously interpret the present recovery of ∆14C to near its pre bomb test value as evidence that atmospheric 14C concentration has returned to its earlier value. From this they reach further incorrect conclusions about the fate of anthropogenic CO2 introduced into the atmosphere by fossil fuel burning. An estimate of the true time dependence of atmospheric 14C concentration over the past century, calculated from averaged atmospheric ∆14C and CO2 data is presented. The data show that 14C concentrations remain over 30% above 1950 values, and have begun to increase, even as ∆14C continues to fall. This confirms the prediction of a conventional model of the carbon cycle. The unconventional models of carbon dynamics motivated by the mistake, on the other hand, are excluded by the properly interpreted 14C data.
    VL  - 9
    IS  - 4
    ER  - 

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Author Information
  • Department of Physics and Astronomy, University of Montana, Missoula, USA

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