American Journal of Chemical Engineering
Volume 5, Issue 1, January 2017, Pages: 1-5
Received: Sep. 22, 2016;
Accepted: Jan. 7, 2017;
Published: Feb. 3, 2017
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Mehdi Zarifian Jenadelh, Dpartment of Chemical Engineering, Sirjan Branch, Islamic Azad University, Sirjan, Iran
Farshad Farahbod, Department of Chemical Engineering, Firoozabad Branch, Islamic Azad University, Firoozabad, Iran
The use of multistage, fluidized beds of continuous recycles reveals economically and technically attractive for both adsorption of stack gas SO2 and sequential conversion to elemental sulfur. This paper studies the adsorption process behavior of SO2 removal in one bed reactor which is filled with zinc oxide nano catalysts. The performance of catalytic bed is analyzed experimentally and theoretically by measuring the rate of mass transfer, NA, in this work. Sulfur elimination from gas is the major purpose of the handled experiments. The specific surface area (15, 20 and 25 m2/m3) as a effective parameter on mass transfer area and the particle diameter (40, 60 and 80 nm) as feed driving force on the amount of NA are evaluated.
Mehdi Zarifian Jenadelh,
Empirical Study of Treatment of Sour Gas by New Technology, American Journal of Chemical Engineering.
Vol. 5, No. 1,
2017, pp. 1-5.
Copyright © 2017 Authors retain the copyright of this article.
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L. Carlos, G. Isabel, B. Irene, D. Luis I,. R. Luis M. Experimental study of SO2 and NOx emissions in fluidized bed oxy-fuel combustion. Fuel Process Techno., 2013; 106: 587–594.
M. de las Obras-Loscertales, A. Rufas, L. F. de Diego, F. García-Labiano, P. Gayán, A. Abad, J. Adánez, Effects of Temperature and Flue Gas Recycle on the SO2 and NOx Emissions in an Oxy-fuel Fluidized Bed Combustor, Energy Procedia., 2013; 37: 1275-1282.
W. Kaewboonsong, V. I. Kuprianov, N. Chovichien, Minimizing fuel and environmental costs for a variable-load power plant (co-) firing fuel oil and natural gas: Part 1. Modeling of gaseous emissions from boiler units, Fuel Processing Technology, 2006; 87: 1085-1094
A. Irabien, Environmental and economic evaluation of SO2 recovery in a ceramic hollow fibre membrane contactor. Chem Eng Process: Process Inten., 2012; 52: 151-154.
H. Wang, Sh. Li, F. Lai, B. Wang, Computational Model of Greenhouse Gas Emissions of Power Station boiler Considering Desulphurization, Physics Procedia, 2012; 24: 44-49.
D. L. Stern, K. E. Nariman, J. S Buchanan, N. A. Bhore, D. L. Johnson, R. K. Grasselli, The Mobil Oil SOx Treatment Process (MOST). Catalytic removal of SOx and H2S from refinery tail gas, Catalysis Today, 2000; 55: 311-316.
W. Zhou, C. S. Zhao, L. B. Duan, XP. Chen, C. Liang, Two-dimensional computational fluid dynamics simulation of nitrogen and sulfur oxides emissions in a circulating fluidized bed combustor. Chem. Eng. J., 2011; 173: 564-573.
D. Eow, S. John, Recovery of sulfur from sour acid gas: A review of the technology Environmental Progress. Americ. Institut. Chem. Eng., 2002; 21: 143-162.
D. Kunii, O. Levenspiel, Fluidization engineering. First edition. New York: Wiley; 1991.
JF. Davidson, Fluidization. First edition. USA: Academic Press; 1991.
D. Green, R. Perry. Perry's Chemical Engineers' Handbook. 8th edition, USA: Mc Graw Hill; 2007.
W. Ch. Yang. Handbook of Fluidization and Fluid-Particle Systems. First edition. USA: Taylor & Francis; 2003.
L. Davidson, Jr Amick, H. Erwin, Formation of gas bubbles at horizontal orifices. AIChE J 2004; 2: 337–342.
M. Uzi. Principles of chemical reactor analysis and design. second edition. New York: Wiley; 2009.
O. Levenspiel, Chemical Reaction Engineering. 3th Ed. New York: Wiley; 1999.
W. J. Reagan, F. M. Dautzenberg, Catalyst Analysis Using Syn- chrotron X-Ray Microscopy, Nucl. Instrum. Methods Phys. Res., 1991; 56/57: 427-432.