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Parametric Investigation of De-Sulfurization Process for Sour Gas; Introduction of Novel System

Received: 7 January 2017    Accepted: 17 January 2017    Published: 27 February 2017
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Abstract

Many different processes are used to treat raw natural gas to pipeline quality. The sulfur is commonly present as an impurity in fossil fuels. Magnetic field is applied in a fluidized bed which contains nano activated carbon to investigate hydrogen sulfide elimination, in this paper. Sulfur removal in this way is presented experimentally and theoretically. The rate of mass transfer is introduced as function of gas temperature, amount of balls covered by nano carbon tubes, initial concentration of hydrogen sulfide, gas flow rate and also, magnetic field. The experimental data are presented and compared with the model results. The effect of hydrogen sulfide in the inlet sour gas on the mass flow rate in investigated in this paper. In addition, the effect of porosity percentage of catalytic bed on the hydrogen sulfide content of outlet gas is evaluated in this paper. The outlet concentration below 4 ppm is acceptable result due to commercial rules. The experimental data are in higher values of hydrogen sulfide comparing with the ones from modeling data.

Published in International Journal of Oil, Gas and Coal Engineering (Volume 5, Issue 1)
DOI 10.11648/j.ogce.20170501.11
Page(s) 1-4
Creative Commons

This is an Open Access article, distributed under the terms of the Creative Commons Attribution 4.0 International License (http://creativecommons.org/licenses/by/4.0/), which permits unrestricted use, distribution and reproduction in any medium or format, provided the original work is properly cited.

Copyright

Copyright © The Author(s), 2024. Published by Science Publishing Group

Keywords

Nano, Hydrogen Sulfide, Flow, Field, Temperature

References
[1] G. J. McLachlan, D. Peel, Finite Mixture Models, Wiley Series in Probability and Statistics, A Wiley-Interscience Publication, 2000.
[2] P. D. Tennis, H. M. Jennings, A model for two types of calcium silicate hydrate in the microstructure of Portland cement pastes, Cem. Concr. Res. 30 (2000) 855–863.
[3] J. Goldstein, Scanning Electron Microscopy and X-ray Microanalysis, Springer, New York, 2008.
[4] M. Miller, Ch. Bobko, M. Vandamme, F.-J. Ulm, “Surface roughness criteria for cement paste nanoindentation”, Cem. Concr. Res. 38 (4) (2011) 467–476.
[5] E. R. Buckle, H. F. W. Taylor, The hydration of tricalcium and β-dicalcium silicates in pastes under normal and steam curing conditions, J. Appl. Chem. 9 (1959) 163–172.
[6] H. F. W. Taylor, The steam curing of Portland cement products, in: H. F. W. Taylor (Ed.), The Chemistry of Cements, vol. 1, Academic Press, London, 1964, pp. 417–432.
[7] G. L. Kalousek, High-temperature curing of concrete under high pressure, Proceedings of the Fifth International Symposium on the Chemistry of Cement, Tokyo, Session III-5, 1964, pp. 523–539.
[8] S. Chatterji, CaO/SiO2 mole ratio of calcium silicate hydrate in fully hydrated tricalcium silicate paste, Cem. Concr. Res. 10 (6) (1980) 783–787.
[9] H. F. W. Taylor, Chemistry of cement hydration, 8th International Congress on the Chemistry of Cement, vol. 1, 1986, pp. 82–110.
[10] H. S. Wong, N. R. Buenfeld, Monte Carlo simulation of electron–solid interactions in cement-based materials, Cem. Concr. Res. 36 (2006) 1076–1082.
[11] M. Abuhaikal, Nano-chemomechanical assessment of rice husk ash cement by wavelength dispersive spectroscopy and nanoindentation, (MSc Thesis) Massachusetts Institute of Technology, 2011.
[12] Mohammad Mahdi Ghiasi, Initial estimation of hydrate formation temperature of sweet natural gases based on new empirical correlation, Journal of Natural Gas Chemistry, Volume 21, Issue 5, September 2012, Pages 508-512.
[13] J. M. Sánchez, M. Maroño, D. Cillero, L. Montenegro, E. Ruiz, Laboratory- and bench-scale studies of a sweet water–gas-shift catalyst for H2 and CO2 production in pre-combustion CO2 capture, Fuel, Volume 114, December 2013, Pages 191-198.
[14] Leila Aliouane, Sid-Ali Ouadfeul, Sweet Spots Discrimination in Shale Gas Reservoirs Using Seismic and Well-logs Data. A Case Study from the Worth Basin in the Barnett Shale,Energy Procedia, Volume 59, 2014, Pages 22-27
[15] Vasileios Pothakos, Clarice Nyambi, Bao-Yu Zhang, Antonios Papastergiadis, Bruno De Meulenaer, Frank Devlieghere, Spoilage potential of psychrotrophic lactic acid bacteria (LAB) species: Leuconostoc gelidum subsp. gasicomitatum and Lactococcus piscium, on sweet bell pepper (SBP) simulation medium under different gas compositions. International Journal of Food Microbiology, Volume 178, 16 May 2014, Pages 120-129
[16] Chunfang Cai, Wenxian He, Lei Jiang, Kaikai Li, Lei Xiang, Lianqi Jia Petrological and geochemical constraints on porosity difference between Lower Triassic sour- and sweet-gas carbonate reservoirs in the Sichuan Basin,Marine and Petroleum Geology, Volume 56, September 2014, Pages 34-50
[17] Azad Jarrahian, Ehsan Heidaryan, A new cubic equation of state for sweet and sour natural gases even when composition is unknown. Fuel, Volume 134, 15 October 2014, Pages 333-342.
[18] Di Cai, Zhen Chang, Lili Gao, Changjing Chen, Yuanpu Niu, Peiyong Qin, Zheng Wang, Tianwei Tan. Acetone–butanol–ethanol (ABE) fermentation integrated with simplified gas stripping using sweet sorghum bagasse as immobilized carrier. Chemical Engineering Journal, Volume 277, 1 October 2015, Pages 176-185
[19] L. Carlos, G. Isabel, B. Irene, D. Luis I,. R. Luis M. Experimental study of SO2 and NOx emissions in fluidized bed oxy-fuel combustion. Fuel Process Techno., 2013; 106: 587–594.
[20] M. de las Obras-Loscertales, A. Rufas, L. F. de Diego, F. García-Labiano, P. Gayán, A. Abad, J. Adánez, Effects of Temperature and Flue Gas Recycle on the SO2 and NOx Emissions in an Oxy-fuel Fluidized Bed Combustor, Energy Procedia., 2013; 37: 1275-1282.
[21] W. Kaewboonsong, V. I. Kuprianov, N. Chovichien, Minimizing fuel and environmental costs for a variable-load power plant (co-)firing fuel oil and natural gas: Part 1. Modeling of gaseous emissions from boiler units, Fuel Processing Technology, 2006; 87: 1085-1094
[22] A. Irabien, Environmental and economic evaluation of SO2 recovery in a ceramic hollow fibre membrane contactor. Chem Eng Process: Process Inten., 2012; 52: 151-154.
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  • APA Style

    Somayyeh Fazeli, Farshad Farahbod. (2017). Parametric Investigation of De-Sulfurization Process for Sour Gas; Introduction of Novel System. International Journal of Oil, Gas and Coal Engineering, 5(1), 1-4. https://doi.org/10.11648/j.ogce.20170501.11

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    ACS Style

    Somayyeh Fazeli; Farshad Farahbod. Parametric Investigation of De-Sulfurization Process for Sour Gas; Introduction of Novel System. Int. J. Oil Gas Coal Eng. 2017, 5(1), 1-4. doi: 10.11648/j.ogce.20170501.11

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    AMA Style

    Somayyeh Fazeli, Farshad Farahbod. Parametric Investigation of De-Sulfurization Process for Sour Gas; Introduction of Novel System. Int J Oil Gas Coal Eng. 2017;5(1):1-4. doi: 10.11648/j.ogce.20170501.11

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  • @article{10.11648/j.ogce.20170501.11,
      author = {Somayyeh Fazeli and Farshad Farahbod},
      title = {Parametric Investigation of De-Sulfurization Process for Sour Gas; Introduction of Novel System},
      journal = {International Journal of Oil, Gas and Coal Engineering},
      volume = {5},
      number = {1},
      pages = {1-4},
      doi = {10.11648/j.ogce.20170501.11},
      url = {https://doi.org/10.11648/j.ogce.20170501.11},
      eprint = {https://article.sciencepublishinggroup.com/pdf/10.11648.j.ogce.20170501.11},
      abstract = {Many different processes are used to treat raw natural gas to pipeline quality. The sulfur is commonly present as an impurity in fossil fuels. Magnetic field is applied in a fluidized bed which contains nano activated carbon to investigate hydrogen sulfide elimination, in this paper. Sulfur removal in this way is presented experimentally and theoretically. The rate of mass transfer is introduced as function of gas temperature, amount of balls covered by nano carbon tubes, initial concentration of hydrogen sulfide, gas flow rate and also, magnetic field. The experimental data are presented and compared with the model results. The effect of hydrogen sulfide in the inlet sour gas on the mass flow rate in investigated in this paper. In addition, the effect of porosity percentage of catalytic bed on the hydrogen sulfide content of outlet gas is evaluated in this paper. The outlet concentration below 4 ppm is acceptable result due to commercial rules. The experimental data are in higher values of hydrogen sulfide comparing with the ones from modeling data.},
     year = {2017}
    }
    

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  • TY  - JOUR
    T1  - Parametric Investigation of De-Sulfurization Process for Sour Gas; Introduction of Novel System
    AU  - Somayyeh Fazeli
    AU  - Farshad Farahbod
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    PY  - 2017
    N1  - https://doi.org/10.11648/j.ogce.20170501.11
    DO  - 10.11648/j.ogce.20170501.11
    T2  - International Journal of Oil, Gas and Coal Engineering
    JF  - International Journal of Oil, Gas and Coal Engineering
    JO  - International Journal of Oil, Gas and Coal Engineering
    SP  - 1
    EP  - 4
    PB  - Science Publishing Group
    SN  - 2376-7677
    UR  - https://doi.org/10.11648/j.ogce.20170501.11
    AB  - Many different processes are used to treat raw natural gas to pipeline quality. The sulfur is commonly present as an impurity in fossil fuels. Magnetic field is applied in a fluidized bed which contains nano activated carbon to investigate hydrogen sulfide elimination, in this paper. Sulfur removal in this way is presented experimentally and theoretically. The rate of mass transfer is introduced as function of gas temperature, amount of balls covered by nano carbon tubes, initial concentration of hydrogen sulfide, gas flow rate and also, magnetic field. The experimental data are presented and compared with the model results. The effect of hydrogen sulfide in the inlet sour gas on the mass flow rate in investigated in this paper. In addition, the effect of porosity percentage of catalytic bed on the hydrogen sulfide content of outlet gas is evaluated in this paper. The outlet concentration below 4 ppm is acceptable result due to commercial rules. The experimental data are in higher values of hydrogen sulfide comparing with the ones from modeling data.
    VL  - 5
    IS  - 1
    ER  - 

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Author Information
  • Department of Chemical Engineering, Sirjan Branch, Islamic Azad University, Sirjan, Iran

  • Department of Chemical Engineering, Firoozabad Branch, Islamic Azad University, Firoozabad, Iran

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